If you want to play your iTunes songs on an Android phone, here's what you need to do. First, download Google’s Music app to your phone from the Google Play Store (your phone might have come. If you have a large iTunes library, then the manual way will take too much time to copy music files from iTunes media folder to your Android device. Another option is to use iTunes to Android Transfer. It offers an one-click way to transfer iTunes music and playlist to Android device. Download, install and run iTunes to Android Transfer on your PC. Can't I Just Plug in My Android Phone and Transfer Music with iTunes? No way. Apple goes to great lengths to ensure iTunes only works with Apple products. It would be great if iTunes could sync music with devices like Android smartphones, but this isn't on Apple's 21st century to-do list. Jul 27, · However, there are several ways you can easily transfer your music collection to your Android smartphone or tablet. Google’s Music Manager application even integrates with your iTunes music library, automatically copying your music to the cloud so you can stream it from anywhere and easily download it to your Android slicelive.com: Chris Hoffman.